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Effects of elastic heterogeneity and anisotropy on the morphology of self-assembled epitaxial quantum dots

机译:弹性非均匀性和各向异性对聚丙烯酰胺形态的影响   自组装外延量子点

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摘要

Epitaxial self-assembled quantum dots (SAQDs) are of both technological andfundamental interest, but their reliable manufacture still presents a technicalchallenge. To better understand the formation, morphology and ordering ofepitaxial self-assembled quantum dots (SAQDs), it is essential to have anaccurate model that can aid further experiments and predict the trends in SAQDformation. SAQDs form because of the destabilizing effect of elastic mismatchstrain, but most analytic models and some numerical models of SAQD formationeither assume an elastically homogeneous anisotropic film-substrate system orassume an elastically heterogeneous isotropic system. In this work, we performthe full film-substrate elastic calculation. Then we incorporate the elasticitycalculation into a stochastic linear growth model. We find that usinghomogeneous elasticity can cause errors in the elastic energy density as largeas 26%, and for typical modeling parameters lead to errors of about 11% in theestimated value of average dot spacing. We also quantify the effect of elasticheterogeneity on the order estimates of SAQDs and confirm previous finding onthe possibility of order enhancement by growing a film near the critical filmheight.
机译:外延自组装量子点(SAQD)既具有技术意义,也具有根本的意义,但是其可靠的制造仍然提出了技术挑战。为了更好地理解外延自组装量子点(SAQD)的形成,形态和有序性,至关重要的是要有一个准确的模型来帮助进一步的实验并预测SAQD形成的趋势。 SAQD的形成是由于弹性失配应变的去稳定作用,但是SAQD形成的大多数分析模型和一些数值模型要么假设弹性均质各向异性膜-基底系统,要么假定弹性异质性各向同性系统。在这项工作中,我们执行完整的薄膜-基材弹性计算。然后,我们将弹性计算纳入随机线性增长模型。我们发现,使用均匀弹性会导致弹性能量密度的误差高达26%,并且对于典型的建模参数,平均点间距的估计值会导致约11%的误差。我们还量化了弹性异质性对SAQD阶数估计的影响,并确认了先前的发现,即通过在临界膜高附近生长膜来增强阶数的可能性。

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